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Published online by Cambridge University Press: 15 February 2011
Resonant optical excitation of fractal clusters generates dipolar eigenmodes which are extremely localized within areas much smaller than the wavelength. The localization occurs due to the fractal morphology and accounts for the very high local fields leading to the huge enhancement of various optical effects. In particular, Rayleigh and Raman light scattering and, especially, nonlinear optical processes, such as 2-photon photoemission and degenerate four-wave mixing, are strongly enhanced in fractal clusters. The spatial distribution of the modes shows the frequency and polarization selectivity.