Published online by Cambridge University Press: 15 February 2011
Radiation effects studies in both glass and glass ceramic nuclear waste forms have identified a rare-earth titanate phase of the general formula (RE) 2Ti207 which is capable of acting as a host phase for actinides.1,2 Ringwood and co-workers3 have also proposed a structurally similar phase, zirconolite (CaZrTi2 07), as one of the primary host phases in the SYNROC waste form. Data from these and other previous studies, as well as mineralogical information available on these titanate phases, have not provided an unambiguous interpretation of the effects of radiation damage relative to nuclear waste forms. This paper reports new laboratory data concerning radiation damage effects in both of these phases.
This work was supported by the U.S. Department of Energy under contract DE-AC06-76RLO 1830.