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Published online by Cambridge University Press: 22 February 2011
We investigated the magnetic excitations in polycrystalline samples of hard magnet related compounds DyFe4Al8 and DyMn4Al8 by neutron spectroscopy. For both compounds the magnetic spectra at energies below 40 meV are dominated by the response of the Dy3+ ions. In DyMn4Al8 we observed pure crystal-field transitions within the Dy3+ J=15/2 ground multiplet which is split into 8 doublets under the low point-group symmetry of 4/mmm. In DyFe4Al8 the Dy crystal-field-split states are perturbed by the molecular fields of the ordered Fe sublattice.
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