Phenomenology of Polymer Solution Dynamics

George D. J. Phillies

doi:10.1017/CBO9780511843181

Presenting a completely new approach to examining how polymers move in non-dilute solution, this book focuses on experimental facts, not theoretical speculations, and concentrates on polymer solutions, not dilute solutions or polymer melts. From centrifugation and solvent dynamics to viscosity and diffusion, experimental measurements and their quantitative representations are the core of the discussion. The book reveals several experiments never before recognized as revealing polymer solution properties. A novel approach to relaxation phenomena accurately describes viscoelasticity and dielectric relaxation and how they depend on polymer size and concentration. Ideal for graduate students and researchers interested in the properties of polymer solutions, the book covers real measurements on practical systems, including the very latest results. Every significant experimental method is presented in considerable detail, giving unprecedented coverage of polymers in solution.

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Contents

Frontmatter
pp i-vi
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Contents
pp vii-xii
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Preface
pp xiii-xvi
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1 - Introduction
pp 1-9
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2 - Sedimentation
pp 10-29
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3 - Electrophoresis
pp 30-68
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4 - Quasielastic light scattering and diffusion
pp 69-93
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5 - Solvent and small-molecule motion
pp 94-115
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6 - Segmental diffusion
pp 116-133
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7 - Dielectric relaxation and chain dimensions
pp 134-170
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8 - Self- and tracer diffusion
pp 171-217
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9 - Probe diffusion
pp 218-286
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10 - Dynamics of colloids
pp 287-319
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11 - The dynamic structure factor
pp 320-354
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12 - Viscosity
pp 355-396
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13 - Viscoelasticity
pp 397-444
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14 - Nonlinear viscoelastic phenomena
pp 445-458
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15 - Qualitative summary
pp 459-474
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16 - Phenomenology
pp 475-493
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17 - Afterword: hydrodynamic scaling model for polymer dynamics
pp 494-498
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Index
pp 499-509
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Phenomenology of Polymer Solution Dynamics

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Contents

Frontmatter
pp i-vi

Contents
pp vii-xii

Preface
pp xiii-xvi

1 - Introduction
pp 1-9

2 - Sedimentation
pp 10-29

3 - Electrophoresis
pp 30-68

4 - Quasielastic light scattering and diffusion
pp 69-93

5 - Solvent and small-molecule motion
pp 94-115

6 - Segmental diffusion
pp 116-133

7 - Dielectric relaxation and chain dimensions
pp 134-170

8 - Self- and tracer diffusion
pp 171-217

9 - Probe diffusion
pp 218-286

10 - Dynamics of colloids
pp 287-319

11 - The dynamic structure factor
pp 320-354

12 - Viscosity
pp 355-396

13 - Viscoelasticity
pp 397-444

14 - Nonlinear viscoelastic phenomena
pp 445-458

15 - Qualitative summary
pp 459-474

16 - Phenomenology
pp 475-493

17 - Afterword: hydrodynamic scaling model for polymer dynamics
pp 494-498

Index
pp 499-509

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