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  3. Nonlinear Optical Polarization Analysis in Chemistry and Biology
  • Cited by 22
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    • Publisher:
      Cambridge University Press
      Publication date:
      May 2017
      March 2017
      ISBN:
      9781139019026
      9780521519083
      DOI:
      https://doi.org/10.1017/9781139019026
      Dimensions:
      (247 x 174 mm)
      Weight & Pages:
      1.13kg, 456 Pages
      Dimensions:
      Weight & Pages:
      • Subjects:
      Optics, Optoelectronics and Photonics, Physics and Astronomy, Engineering, Physical Chemistry, Atomic Physics, Molecular Physics and Chemical Physics, Materials Science
      Product:
      Materials Research Society
      Series:
      Cambridge Molecular Science
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    Subjects:
    Optics, Optoelectronics and Photonics, Physics and Astronomy, Engineering, Physical Chemistry, Atomic Physics, Molecular Physics and Chemical Physics, Materials Science
    Product:
    Materials Research Society
    Series:
    Cambridge Molecular Science
    Information

    Book description

    This rigorous yet accessible guide presents a molecular-based description of nonlinear optical polarization analysis of chemical and biological assemblies. It includes discussion of the most common nonlinear optical microscopy and interfacial measurements used for quantitative analysis, specifically second harmonic generation (SHG), two-photon excited fluorescence (2PEF), vibrational sum frequency generation (SFG), and coherent anti-Stokes Raman spectroscopy/stimulated Raman spectroscopy (CARS/SRS). A linear algebra mathematical framework is developed, allowing step-wise systematic connections to be made between the observable measurements and the molecular response. Effects considered include local field corrections, the molecular orientation distribution, rotations between the molecular frame, the local frame and the laboratory frame, and simplifications from molecular and macromolecular symmetry. Specific examples are provided throughout the book, working from the common and relatively simple case studies through to the most general scenarios.

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